The results are likely to be announced by 7 pm.
Gandhi also spoke about the importance of voting for the vice-president, saying, "Today everyone came together to vote for what they thought was the national good".
The total strength of the Lok Sabha and the Rajya Sabha is 790.
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Naidu yet again kicked up a political storm when he said seeking loan waivers had become a "fashion".
"I am very humbled". The JD (U) broke ties with "mahagathbandhan" and joined hands with the Bharatiya Janata Party (BJP) to form a new government in Bihar, but made a decision to vote for Gandhi.
Vice President is the second highest constitutional post in India and is also the "ex-officio" Chairperson of the Rajya Sabha, upper chamber of Parilament. Prime Minister Narendra Modi's administation has a majority in the lower house but trails in 245-member upper house.
Gopalkrishna Gandhi is the grandson of Mahatma Gandhi.
He further said Naidu will be one of the finest vice presidents and will conduct Rajya Sabha by taking everyone into confidence. Apart from being the deputy to President Ram Nath Kovind, Naidu will also be the Chairman of Rajya Sabha. Naidu hit the national scene when he was one of the prominent opposition spokespersons along with S Jaipal Reddy, who was then in Janata Party, during the campaign by NT Rama Rao after his dismissal as the Andhra Pradesh chief minister by Indira Gandhi in the 1980s. The voting to elect the next Vice President will be held tomorrow August 5th. Gandhi, the former Governor of West Bengal and a diplomat, was supported by the Congress, the Left parties, the Nationalist Congress Party, the Dravida Munetra Kazhagam, the Trinamool Congress, the Bahujan Samaj Party and the National Conference. If he wins or rather when he wins, he will be succeeding Mohammad Hamid Ansari, whose term ends on August 10. During NDA-1 government, BJP lacked the number to install a candidate for the Presidential post. Of this number, 40 MPs, from the Biju Janata Dal and the Janata Dal (U) chose to shift their votes from the NDA to the Opposition candidate for the vice-presidential polls. He appealed to NDA MPs to vote for Naidu in the election of Vice President. Added to this were 10 nominated members, most of whom were expected to vote for Mr Naidu.